Abstract: Dicyanoacetylene has not been observed so far in the gas phase in Titan’s atmosphere but this molecule is still on the list of the detected species, on the basis of the correspondence between a solid phase feature measured at 478 cm1 in the laboratory and a spectral feature observed by Voyager. In this work, the infrared spectrum of gaseous C4N2 has been investigated to improve our knowledge of the band intensities and the line parameters for this molecule. Results of previously investigated bands have been revised and the intensity of the m9 band at 107 cm1, measured for the first time, was found to be the strongest absorption in the whole infrared domain...